Počet záznamů: 1  

A novel glue attachment approach for precise anchoring of hydrophilic EGCG to enhance the separation performance and antifouling properties of PVDF membranes

  1. 1.
    SYSNO ASEP0571686
    Druh ASEPJ - Článek v odborném periodiku
    Zařazení RIVJ - Článek v odborném periodiku
    Poddruh JČlánek ve WOS
    NázevA novel glue attachment approach for precise anchoring of hydrophilic EGCG to enhance the separation performance and antifouling properties of PVDF membranes
    Tvůrce(i) Zhuang, G. (TW)
    Wang, L. (TW)
    Lin, Y. (TW)
    Li, J. (TW)
    Setničková, Kateřina (UCHP-M) RID, ORCID, SAI
    Tseng, H. (TW)
    Číslo článku142585
    Zdroj.dok.Chemical Engineering Journal. - : Elsevier - ISSN 1385-8947
    Roč. 464, May15 (2023)
    Poč.str.14 s.
    Jazyk dok.eng - angličtina
    Země vyd.NL - Nizozemsko
    Klíč. slovahydrophilic surface modification ; reclaimed rubber ; epigallocatechin gallate ; hydrogen bond
    Obor OECDChemical process engineering
    Způsob publikováníOpen access s časovým embargem (16.05.2025)
    Institucionální podporaUCHP-M - RVO:67985858
    UT WOS000963764600001
    EID SCOPUS85151024968
    DOI10.1016/j.cej.2023.142585
    AnotaceA novel glue attachment approach was proposed to form a durable hydration layer on a hydrophobic PVDF hollow fiber membrane (PVDF HFM) surface to improve its hydrophilicity and antifouling ability during wastewater filtration. The functional glue was synthesized from reclaimed styrene butadiene rubber (SBR) and a hydroxyl group was created with an epoxidation reaction (ESBR). The hydrophilic epigallocatechin-s-gallate (EGCG) was then precisely anchored via hydrogen bonding with multiple phenolic hydroxyl groups in the ESBR without penetrating into the inner matrix of the PVDF to prevent flux decline. The hydrophilicity of the PVDF membrane increased drastically and the water contact angle decreased from 62.7 degrees to 45.1 degrees with only a 25% decline in the pure water flux. Furthermore, due to precise anchoring of the EGCG, the modified EGCG-ESBR/PVDF membrane showed a higher pure water flux (110.6 L m(-2) h(-1)) and much higher BSA and oil (kerosene) rejection rates (approximately 94.5% and 99.5%, respectively) compared to membranes directly coated with EGCG (EGCG-PVDF). Moreover, the modified membrane also showed higher water flux recovery after multiple filtration cycles. This promising and efficient hydrophilic modification suggests great potential for application of the eco-friendly material in wastewater treatment.
    PracovištěÚstav chemických procesů
    KontaktEva Jirsová, jirsova@icpf.cas.cz, Tel.: 220 390 227
    Rok sběru2024
    Elektronická adresahttps://hdl.handle.net/11104/0342741
Počet záznamů: 1  

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