0525154 - ÚPT 2021 RIV US eng J - Článek v odborném periodiku
Valero, A.C. - Kislov, D. - Gurvitz, E.A. - Shamkhi, H. - Pavlov, A.A. - Redka, D. - Yankin, S. - Zemánek, Pavel - Shalin, A.S.
Nanovortex-Driven All-Dielectric Optical Diffusion Boosting and Sorting Concept for Lab-on-a-Chip Platforms.
Advanced Science. Roč. 7, č. 11 (2020), č. článku 1903049. ISSN 2198-3844. E-ISSN 2198-3844
Grant CEP: GA ČR(CZ) GA19-17765S; GA TA ČR TE01020233
Institucionální podpora: RVO:68081731
Klíčová slova: all-dielectric nanophotonics * lab-on-a-chip platforms * nanofluidics * optomechanical manipulations * spin-orbit couplings
Obor OECD: Optics (including laser optics and quantum optics)
Impakt faktor: 16.806, rok: 2020
Způsob publikování: Open access
Web výsledku:
https://onlinelibrary.wiley.com/doi/full/10.1002/advs.201903049
DOI: https://doi.org/10.1002/advs.201903049

The ever-growing field of microfluidics requires precise and flexible control over fluid flows at reduced scales. Current constraints demand a variety of controllable components to carry out several operations inside microchambers and microreactors. In this context, brand-new nanophotonic approaches can significantly enhance existing capabilities providing unique functionalities via finely tuned light-matter interactions. A concept is proposed, featuring dual on-chip functionality: boosted optically driven diffusion and nanoparticle sorting. High-index dielectric nanoantennae is specially designed to ensure strongly enhanced spin-orbit angular momentum transfer from a laser beam to the scattered field. Hence, subwavelength optical nanovortices emerge driving spiral motion of plasmonic nanoparticles via the interplay between curl-spin optical forces and radiation pressure. The nanovortex size is an order of magnitude smaller than that provided by conventional beam-based approaches. The nanoparticles mediate nanoconfined fluid motion enabling moving-part-free nanomixing inside a microchamber. Moreover, exploiting the nontrivial size dependence of the curled optical forces makes it possible to achieve precise nanoscale sorting of gold nanoparticles, demanded for on-chip separation and filtering. Altogether, a versatile platform is introduced for further miniaturization of moving-part-free, optically driven microfluidic chips for fast chemical analysis, emulsion preparation, or chemical gradient generation with light-controlled navigation of nanoparticles, viruses or biomolecules.

Trvalý link: http://hdl.handle.net/11104/0309357