Influence of In-induced resonant level on the normal-state and superconducting properties of Sn1.03Te

Shantanu Misra, Bartlomiej Wiendlocha, Janusz Tobola, Petr Levinský, Jiří Hejtmánek, Sylvie Migot, Jaafar Ghanbaja, Anne Dauscher, Bertrand Lenoir, and Christophe Candolfi
Phys. Rev. B 106, 075205 – Published 29 August 2022

Abstract

Normal-state transport properties (2–300 K) of the polycrystalline series Sn1.03δxInxTe (0x0.07; δ0.0025) were investigated by means of electrical resistivity, thermopower, Hall effect, and thermal conductivity measurements. The distortion of the valence-band structure by the In-induced resonant level (RL) has a profound influence on the evolution of the normal-state properties with x and on the emergence of superconductivity evidenced by specific-heat measurements down to 0.35 K. In addition to a nearly 40-fold increase in the residual electrical resistivity ρ0 on going from x=0.0 to 0.05, the thermopower α shows a nonlinear, complex behavior as a function of both temperature and x. While Hall measurements indicate a dominant holelike response across the entire composition and temperature ranges, α changes sign below about 100 K and remains negative down to 5 K for 0.0015x0.0045. Additional measurements under magnetic fields μ0H of up to 14 T further shows that α(μ0H) gradually shifts towards positive values, suggestive of a dominant holelike contribution to α. Superconductivity emerges for x=0.02 at a critical temperature Tc=0.67 K, with Tc increasing with x to reach 1.73 K for x=0.07. The variations in the superconducting parameters with x, notably the specific-heat jump at Tc, confirm the results reported in prior studies and suggests a nontrivial role of the RL on the electron-phonon coupling strength. The striking similarities between this series and the canonical resonant system Pb1xTlxTe provide an excellent experimental opportunity to gain a deeper understanding of the close interplay between resonant level, anomalous transport properties, and superconductivity.

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  • Received 24 November 2021
  • Revised 3 May 2022
  • Accepted 5 August 2022

DOI:https://doi.org/10.1103/PhysRevB.106.075205

©2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Shantanu Misra1, Bartlomiej Wiendlocha2,*, Janusz Tobola2, Petr Levinský3, Jiří Hejtmánek3, Sylvie Migot1, Jaafar Ghanbaja1, Anne Dauscher1, Bertrand Lenoir1, and Christophe Candolfi1,†

  • 1Institut Jean Lamour, UMR 7198 CNRS – Université de Lorraine, 2 allée André Guinier-Campus ARTEM, BP 50840, 54011 Nancy Cedex, France
  • 2Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, Aleja Mickiewicza 30, 30-059 Krakow, Poland
  • 3Institute of Physics, Czech Academy of Sciences, Cukrovarnická 10, 162 00, Praha 6, Czech Republic

  • *wiendlocha@fis.agh.edu.pl
  • christophe.candolfi@mines-nancy.univ-lorraine.fr

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Vol. 106, Iss. 7 — 15 August 2022

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