Evidence for spin-glass ground state in fluorite-defect Er2Zr2O7 single crystals

K. Vlášková, R. H. Colman, P. Proschek, J. Čapek, and M. Klicpera
Phys. Rev. B 100, 214405 – Published 2 December 2019

Abstract

We present the preparation and characterization of an Er2Zr2O7 single crystal. The material was studied by means of x-ray and neutron diffraction, magnetization, AC susceptibility, and specific heat measurements. The defect-fluorite type of cubic structure, previously reported as the crystal structure of Er2Zr2O7, is consistent with our x-ray powder diffraction data. The measurements of physical properties were performed in magnetic field applied along principal crystallographic directions. A negligible directional dependence of physical properties is observed at temperatures down to 3 K, and only minor differences can be traced at lower temperatures. A low-temperature anomaly in magnetization and specific heat data and its evolution with applied magnetic field is followed. A frequency-dependent shift of freezing temperature was observed in AC susceptibility. Several origins of the observed anomaly are discussed, leaving a spin-glass state as the most probable explanation.

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  • Received 24 October 2018
  • Revised 28 June 2019

DOI:https://doi.org/10.1103/PhysRevB.100.214405

©2019 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

K. Vlášková1, R. H. Colman1, P. Proschek1, J. Čapek2, and M. Klicpera1

  • 1Charles University, Faculty of Mathematics and Physics, Department of Condensed Matter Physics, Ke Karlovu 5, 12116 Prague 2, Czech Republic
  • 2Institute of Physics ASCR, v.v.i., Na Slovance 2, 182 21 Praha 8, Czech Republic

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Issue

Vol. 100, Iss. 21 — 1 December 2019

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