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Strain-controlled optical absorption in epitaxial ferroelectric BaTiO.sub.3./sub. films

  1. 1.
    SYSNO ASEP0449010
    Document TypeJ - Journal Article
    R&D Document TypeJournal Article
    Subsidiary JČlánek ve WOS
    TitleStrain-controlled optical absorption in epitaxial ferroelectric BaTiO3 films
    Author(s) Chernova, Ekaterina (FZU-D)
    Pacherová, Oliva (FZU-D) RID, ORCID
    Chvostová, Dagmar (FZU-D) RID, SAI, ORCID
    Dejneka, Alexandr (FZU-D) RID, ORCID
    Kocourek, Tomáš (FZU-D) RID, ORCID, SAI
    Jelínek, Miroslav (FZU-D) RID, ORCID
    Tyunina, Marina (FZU-D) ORCID
    Source TitleApplied Physics Letters. - : AIP Publishing - ISSN 0003-6951
    Roč. 106, č. 19 (2015), "192903-1"-"192903-4"
    Number of pages4 s.
    Languageeng - English
    CountryUS - United States
    Keywordsthin-films ; polarization ; evolution ; SrTiO3
    Subject RIVBM - Solid Matter Physics ; Magnetism
    R&D ProjectsGA15-13778S GA ČR - Czech Science Foundation (CSF)
    GA15-15123S GA ČR - Czech Science Foundation (CSF)
    Institutional supportFZU-D - RVO:68378271
    UT WOS000355008100027
    EID SCOPUS84929379829
    DOI10.1063/1.4921083
    AnnotationA lattice strain of 0.3%-1.3% is achieved in epitaxial tetragonal BaTiO3 films grown on (001)-oriented SrTiO3 single-crystal substrates. Our experimental studies of absorption spectra in the range of 0.74-9.0 eV demonstrate that epitaxy produces significant changes in the optical properties of the films compared with those of a reference polydomain BaTiO3 crystal: the absorption edge and the peak at 5 eV strongly blue-shift by 0.2-0.4 eV, the magnitude of the peak at 5 eV drops, and certain spectral features disappear, whereas the absorption peak at 8.5 eV remains unchanged. The observed behavior is attributed to ferroelectric polarization, which is enhanced by epitaxial strain in the films. Our results indicate that epitaxially induced variations of ferroelectric polarization may be used to tailor the optical properties of thin films for photonic and optoelectronic applications.
    WorkplaceInstitute of Physics
    ContactKristina Potocká, potocka@fzu.cz, Tel.: 220 318 579
    Year of Publishing2016
Number of the records: 1  

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