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Luminescence of nanodiamond driven by atomic functionalization: Towards novel detection principles
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SYSNO ASEP 0376576 Document Type J - Journal Article R&D Document Type Journal Article Subsidiary J Článek ve WOS Title Luminescence of nanodiamond driven by atomic functionalization: Towards novel detection principles Author(s) Petráková, V. (CZ)
Taylor, Andrew (FZU-D) RID, ORCID
Kratochvílová, Irena (FZU-D) RID, ORCID, SAI
Fendrych, František (FZU-D) RID, ORCID, SAI
Vacík, Jiří (UJF-V) RID, ORCID, SAI
Kučka, Jan (UJF-V) RID
Štursa, Jan (UJF-V) RID, ORCID
Cígler, Petr (UOCHB-X) RID, ORCID
Ledvina, Miroslav (UOCHB-X) RID
Fišerová, Anna (MBU-M) RID
Kneppo, P. (CZ)
Nesládek, M. (BE)Source Title Advanced Functional Materials - ISSN 1616-301X
Roč. 22, č. 4 (2012), s. 812-819Number of pages 7 s. Language eng - English Country DE - Germany Keywords nanodiamond ; nanoparticles ; luminescent centers ; NV ; surface functionalization ; molecular imaging Subject RIV BM - Solid Matter Physics ; Magnetism R&D Projects KAN200100801 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) KAN301370701 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) KAN400480701 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) CEZ AV0Z10100520 - FZU-D (2005-2011) AV0Z10480505 - UJF-V (2005-2011) AV0Z40550506 - UOCHB-X (2005-2011) AV0Z50200510 - MBU-M (2005-2011) UT WOS 000300447500017 DOI 10.1002/adfm.201101936 Annotation Here we present a novel method for remote monitoring of chemical processes in biological environments based on color changes from photoluminescence of NV centers in ND. We propose to drive the NV luminescence chemically, by alternating the surface electric field developed by interacting atoms and molecules with the diamond surface. We demonstrate this phenomenon on oxidized and hydrogenated ND as well as single crystal diamond containing engineered NV centers to the nm-depth. The hydrogenation of NDs leads to quenching of luminescence related to negatively charged (NV-) centers and this way produces changes in the intensity ratio between NV- (636 nm) to neutral NV0 (575nm) centers. We discuss how the reduction of diamond size increases the magnitude of NV color shift mechanism. Workplace Institute of Physics Contact Kristina Potocká, potocka@fzu.cz, Tel.: 220 318 579 Year of Publishing 2013
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