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Nonradiative electron and energy transfer. Explicit estimation of the influence of coherent and dephasing processes in a vibrational bath on electronic dynamics
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SYSNO ASEP 0333611 Document Type J - Journal Article R&D Document Type Journal Article Subsidiary J Článek ve WOS Title Nonradiative electron and energy transfer. Explicit estimation of the influence of coherent and dephasing processes in a vibrational bath on electronic dynamics Author(s) Menšík, Miroslav (UMCH-V) RID
Král, Karel (FZU-D) RIDSource Title Materials Science-Poland - ISSN 0137-1339
Roč. 27, č. 3 (2009), s. 671-684Number of pages 14 s. Action International Conference on Electrical and Related Properties of Organic Solids /11./ Event date 13.07.2008-17.07.2008 VEvent location Piechowice Country PL - Poland Event type WRD Language eng - English Country PL - Poland Keywords electron-vibrational interaction ; non-adiabatic coupling ; resonant energy transfer Subject RIV CD - Macromolecular Chemistry R&D Projects KAN401770651 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) GA202/07/0643 GA ČR - Czech Science Foundation (CSF) CEZ AV0Z40500505 - UMCH-V (2005-2011) AV0Z10100520 - FZU-D (2005-2011) UT WOS 000272085200007 Annotation A theoretical model is studied of the coupling of several electronic states to a vibrational manifold. In this approach, the vibrational manifold is divided into two subbaths. The first one, a coherent subbath, interacts coherently with electronic states. The second one, a thermalizing subbath, is responsible for relaxation of vibronic energy. In the first step, the thermalizing subbath is projected out, under the assumption of a standard (Markovian) approximation in the interaction picture and the effective dissipative Liouville equation for a coherent vibronic system (electronic states + coherent bath modes) is thus obtained. Workplace Institute of Macromolecular Chemistry Contact Eva Čechová, cechova@imc.cas.cz ; Tel.: 296 809 358 Year of Publishing 2010
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