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Efficient Tar Removal from Biomass Producer Gas at Moderate Temperatures via Steam Reforming on Nickel-based Catalyst
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SYSNO ASEP 0330710 Document Type C - Proceedings Paper (int. conf.) R&D Document Type The record was not marked in the RIV Title Efficient Tar Removal from Biomass Producer Gas at Moderate Temperatures via Steam Reforming on Nickel-based Catalyst Author(s) Vosecký, Martin (UCHP-M)
Kameníková, Petra (UCHP-M) RID, SAI
Pohořelý, Michael (UCHP-M) RID, ORCID, SAI
Skoblia, Sergej (UCHP-M)
Punčochář, Miroslav (UCHP-M) RID, ORCID, SAISource Title Proceedings. - - : -, 2009 - ISBN N Pages s. 862-866 Number of pages 5 s. Action European Biomass Conference and Exhibition /17./ Event date 29.06.2009-03.07.2009 VEvent location Hamburg Country DE - Germany Event type WRD Language eng - English Country DE - Germany Keywords tar removal ; catalytic conversion ; biomass gasification Subject RIV CI - Industrial Chemistry, Chemical Engineering R&D Projects GA104/07/0977 GA ČR - Czech Science Foundation (CSF) 2B08048 GA MŠMT - Ministry of Education, Youth and Sports (MEYS) CEZ AV0Z40720504 - UCHP-M (2005-2011) Annotation The present work deals with tar removal from biomass producer gas by means of a nickel-based catalyst at temperatures about 500 °C. The proposed concept has been firstly verified by the laboratory-scale experiments in which benzene, toluene and naphthalene were chosen as tar model compounds. It has been observed at about 500 °C, GHSV > 25 000 h–1 and H2O/C = 18 mol mol–1 that conversions of all tar model compounds higher than 95 % can be gained. Secondly, experiments with real producer gas have been performed. A side stream of hot raw producer gas was dedusted in the first reactor at temperatures 550–600 °C. Gas was exposed to the chosen-nickel based catalyst at about 500 °C, GHSV = 3360–6000 h–1 and H2O/C = 5–6 mol mol–1. It has been found, that hydrocarbons higher than methane including tar species were decomposed into H2 and CO2. Tar species were effectively decomposed from more than 3 g m–3 to less than 17 mg m–3 which corresponds to conversions higher than 99 %. Workplace Institute of Chemical Process Fundamentals Contact Eva Jirsová, jirsova@icpf.cas.cz, Tel.: 220 390 227 Year of Publishing 2010
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