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Novel Approach to Tar Removal from Biomass Producer Gas by Means of a Nickel-based Catalyst
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SYSNO ASEP 0330704 Document Type C - Proceedings Paper (int. conf.) R&D Document Type Conference Paper Title Novel Approach to Tar Removal from Biomass Producer Gas by Means of a Nickel-based Catalyst Title Odstraňování dehtu na niklovém katalyzátoru z plynu ze zplyňování biomasy Author(s) Vosecký, Martin (UCHP-M)
Kameníková, Petra (UCHP-M) RID, SAI
Pohořelý, Michael (UCHP-M) RID, ORCID, SAI
Skoblia, Sergej (UCHP-M)
Punčochář, Miroslav (UCHP-M) RID, ORCID, SAISource Title Proceedings. - Beijing : Tsingua University Press, 2009 / Yue G. ; Zhang H. ; Zhao C. ; Luo Z. - ISBN 978-7-302-20146-5 Pages s. 740-746 Number of pages 7 s. Action International Conference on Fluidized Bed Combustion /20./ Event date 18.05.2009-21.05.2009 VEvent location Xi’an Country CN - China Event type WRD Language eng - English Country CN - China Keywords catalytic tar removal ; nickel catalyst ; biomass gasification Subject RIV CI - Industrial Chemistry, Chemical Engineering R&D Projects GA104/07/0977 GA ČR - Czech Science Foundation (CSF) 2B08048 GA MŠMT - Ministry of Education, Youth and Sports (MEYS) CEZ AV0Z40720504 - UCHP-M (2005-2011) Annotation The nickel-based catalyst was exposed to the raw gas from gasification of woody biomass with air in a fluidized-bed. Steam reforming reactions led to decomposition of tar and all hydrocarbons higher than CH4 into mainly H2 and CO which further underwent reaction with steam via the water gas shift reaction to CO2. The reforming reactions caused approximately 10-20 % decrease in the lower heating values of the producer gas from the inlet values 5.0–6.5 MJ m-3. The gas yield increased from values 2.4–2.6 m3 kg-1 to values 2.8–3.0 m3 kg-1 on dry biomass basis. The chosen tar removal concept based on combination of dolomite in the fluidized-bed with the secondary catalytic reactor was proved by 20 hours long experiment in which the final tar content below 30 mg m-3 was attained corresponding to more than 97 % tar conversion. Workplace Institute of Chemical Process Fundamentals Contact Eva Jirsová, jirsova@icpf.cas.cz, Tel.: 220 390 227 Year of Publishing 2010
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