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N2O Decomposition over Fe-Ferrierite: Primary and Secondary Reactions with Reducing Agents
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SYSNO ASEP 0322810 Document Type J - Journal Article R&D Document Type Journal Article Subsidiary J Článek ve WOS Title N2O Decomposition over Fe-Ferrierite: Primary and Secondary Reactions with Reducing Agents Title Rozklad N2O na Fe-ferrieritu: primární a sekundární reakce Author(s) Nováková, Jana (UFCH-W) RID
Sobalík, Zdeněk (UFCH-W) RIDSource Title Catalysis Letters - ISSN 1011-372X
Roč. 127, 1-2 (2009), s. 95-100Number of pages 6 s. Language eng - English Country US - United States Keywords N2O decomposition ; reactivity of surface species ; Fe-ferrierite Subject RIV CF - Physical ; Theoretical Chemistry R&D Projects 1ET400400413 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) 1QS400400560 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) CEZ AV0Z40400503 - UFCH-W (2005-2011) UT WOS 000261786400015 DOI 10.1007/s10562-008-9638-7 Annotation The decomposition of N2O either alone or with several reducing agents (CH4, CO, NO and D-2) was followed by temperature-programmed desorption of surface species formed during the reactions. TPD products formed in these "primary" reactions were compared with the TPD products after "secondary" reactions of the same set of reducing agents with the surface species formed during the primary reactions. Changes in TPD products after reactions measured under various conditions were analyzed in detail. These experiments provided a background for studies of the nature and reactivity of surface species formed during N2O reactions over Fe-ferrierite. The relevance of these experimental results to the mechanism of the N2O elimination is discussed. Workplace J. Heyrovsky Institute of Physical Chemistry Contact Michaela Knapová, michaela.knapova@jh-inst.cas.cz, Tel.: 266 053 196 Year of Publishing 2009
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