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Size control of nanoparticles synthesized by pulsed laser ablation in liquids using donut-shaped beams

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    0618796 - FZÚ 2026 RIV DE eng J - Journal Article
    Altakroury, A. R. - Gatsa, Oleksandr - Riahi, F. - Fu, Z.W. - Flimelová, Miroslava - Samokhvalov, A. - Barcikowski, S. - Donate-Buendia, C. - Bulgakov, Alexander V. - Goekce, B.
    Size control of nanoparticles synthesized by pulsed laser ablation in liquids using donut-shaped beams.
    Beilstein Journal of Nanotechnology. Roč. 16, Mar (2025), s. 407-417. ISSN 2190-4286. E-ISSN 2190-4286
    R&D Projects: GA MŠMT(CZ) EH22_008/0004596; GA ČR(CZ) GF22-38449L
    Institutional support: RVO:68378271
    Keywords : beam shaping * cavitation bubble * donut beam * gold nanoparticles * high-entropy alloy nanoparticles * nanoparticle size analysis * yttrium oxide nanoparticles
    OECD category: Nano-materials (production and properties)
    Impact factor: 2.6, year: 2023 ; AIS: 0.472, rok: 2023
    Method of publishing: Open access
    DOI: https://doi.org/10.3762/bjnano.16.31

    The potential to modify the size distribution of nanoparticles synthesized by pulsed laser ablation in liquids is demonstrated using a donut-shaped laser beam. In experiments on pulsed laser ablation in water of gold, yttrium oxide, and high-entropy alloy targets with both Gaussian and donut-shaped beams, we observed a significant reduction in particle size, narrowing of the size distribution width, and an improvement in sphericity when utilizing the donut-shaped laser beam. We performed time-resolved shadowgraph imaging of the laser-induced cavitation bubble, revealing a toroidal structure that overruns the ring-shaped ablation site, compared to the quasi-hemispherical bubble covering the ablation spot produced by the Gaussian beam. Based on this pioneering study, further investigation with higher temporal and spatial resolution are warranted.
    Permanent Link: https://hdl.handle.net/11104/0365731
     
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    Size control of nanoparticles synthesized by pulsed laser ablation in liquids using donut-shaped beams
     
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