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How Nucleobases Rotate When Bonded to a Metal Ion: Detailed View from an ab initio Quantum Chemical Study of a Cytosine Complex of trans-a.sub.2./sub.PT.sup.II./sup..

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    0181281 - UFCH-W 20010202 RIV US eng J - Journal Article
    Šponer, Judit E. - Glahé, F. - Leszczynski, J. - Lippert, B. - Šponer, Jiří
    How Nucleobases Rotate When Bonded to a Metal Ion: Detailed View from an ab initio Quantum Chemical Study of a Cytosine Complex of trans-a2PTII.
    Journal of Physical Chemistry. B. Roč. 105, č. 48 (2001), s. 12171-12179. ISSN 1089-5647
    R&D Projects: GA MŠMT LN00A032
    Institutional research plan: CEZ:AV0Z4040901
    Keywords : ab initio * metaleted base pairs * metal cations
    Subject RIV: CF - Physical ; Theoretical Chemistry
    Impact factor: 3.379, year: 2001

    A systematic quantum-chemical characterization of intrinsic structural and energetical properties of the model nucleobase complex. Special attention has been paid to relative stabilities of the species with head-tail and head-head orientations of the bases and to the interconversion path between them. Present study demostrates that contemporary quantum-chemical calculations capturing the intrinsic gas-phase properties of studied species provide a very useful complement to condensed phase and x-ray studies.
    Permanent Link: http://hdl.handle.net/11104/0077863


     
     

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