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Geometrical and Electronic Structures of the Acetyl Complex Re(bpy)(CO).sub.3./sub.(COCH.sub.3./sub.) and of [M(bpy)(CO).sub.4./sub.](OTf), M=Mn, Re

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    SYSNO ASEP0181037
    Document TypeJ - Journal Article
    R&D Document TypeJournal Article
    Subsidiary JOstatní články
    TitleGeometrical and Electronic Structures of the Acetyl Complex Re(bpy)(CO)3(COCH3) and of [M(bpy)(CO)4](OTf), M=Mn, Re
    Author(s) Scheiring, T. (DE)
    Kaim, W. (DE)
    Fiedler, Jan (UFCH-W) RID, ORCID
    Source TitleJournal of Organometallic Chemistry. - : Elsevier - ISSN 0022-328X
    Roč. 598, č. 1 (2000), s. 136-141
    Languageeng - English
    CountryCH - Switzerland
    Subject RIVCF - Physical ; Theoretical Chemistry CF - Physical ; Theoretical Chemistry
    R&D ProjectsOC D14.20 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    CEZAV0Z4040901 - UFCH-W
    A54/98:Z4-040-9-ii
    AnnotationThe title compounds has been investigated by infrared spectroelectrochemistry to reveal the occupation of the pi*(bpy)MO on one-electron reduction to radical-anion with negligible participation of the pi-accepting acetyl group.Crystal structure analysis of Re(bpy)(CO) 3 (COCH 3 ) revealed a short C-O(acetyl) and long Re-C(acetyl) bond and an orientation of the Re-C(O)CH 3 plane parallel to C 2 axis of coordinated bpy.
    WorkplaceJ. Heyrovsky Institute of Physical Chemistry
    ContactMichaela Knapová, michaela.knapova@jh-inst.cas.cz, Tel.: 266 053 196
    Year of Publishing2001

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