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Effect of the Phase Volume Ratio on the Potential of a Liquid-Membrane Ion-Selective Electrode

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    SYSNO ASEP0101093
    Document TypeJ - Journal Article
    R&D Document TypeJournal Article
    Subsidiary JOstatní články
    TitleEffect of the Phase Volume Ratio on the Potential of a Liquid-Membrane Ion-Selective Electrode
    TitleVliv poměru objemu fází na potenciál iontově selektivní elektrody s kapalnou membránou
    Author(s) Samec, Zdeněk (UFCH-W) RID, ORCID
    Girault, H. H. (CH)
    Source TitleAnalytical Chemistry. - : American Chemical Society - ISSN 0003-2700
    Roč. 76, č. 14 (2004), s. 4150-4155
    Number of pages6 s.
    Languageeng - English
    CountryUS - United States
    Keywordsliquit-membrane ; ion-selective electrode ; two.phase liquid system
    Subject RIVCG - Electrochemistry
    R&D ProjectsME 502 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    CEZAV0Z4040901 - UFCH-W
    AnnotationTwo-phase liquid system IA(w)|IX(o) comprising the interface between the aqueous solution (w) of uni-univalent electrolyte IA and an organic solvent solution (o) of a uni-univalent electrolyte IX with the common cation I+is considered as a simple model of a liquid-membrane ion-selective electrode (ISE). Taking into account the electroneutrality and mass balance conditions, the equilibrium Galvani potential difference (pd) between the aqueous and organic phases. Numeric results corroborate the symbolic expressions derived for the cases when X- and A- are extremely lipophilic and hydrophilic ions, respectively, or when the concentration ratio x is extremely large or small. In contrast to the extraction system, where both electrolytes are initially present in the aqueous phase, the effect of the phase volume ratio on the equilibrium pd in the ISE model is rather weak, unless the counterions X- and A- differ little in their lipophilicity from the target ion I+.
    WorkplaceJ. Heyrovsky Institute of Physical Chemistry
    ContactMichaela Knapová, michaela.knapova@jh-inst.cas.cz, Tel.: 266 053 196
    Year of Publishing2005
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