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Interplay between π-conjugation and exchange magnetism in one-dimensional porphyrinoid polymers
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SYSNO ASEP 0561260 Document Type J - Journal Article R&D Document Type Journal Article Subsidiary J Článek ve WOS Title Interplay between π-conjugation and exchange magnetism in one-dimensional porphyrinoid polymers Author(s) Biswas, K. (ES)
Urbani, M. (ES)
Sánchez-Grande, A. (ES)
Soler Polo, Diego Manuel (FZU-D)
Lauwaet, K. (ES)
Matěj, Adam (FZU-D) ORCID
Mutombo, Pingo (FZU-D) RID, ORCID
Veis, Libor (UFCH-W) RID, ORCID
Brabec, Jiří (UFCH-W) RID, ORCID
Pernal, K. (PL)
Gallego, J. M. (ES)
Miranda, R. (ES)
Écija, D. (ES)
Jelínek, Pavel (FZU-D) RID, ORCID
Torres, T. (ES)
Urgel, J. I. (ES)Number of authors 16 Source Title Journal of the American Chemical Society. - : American Chemical Society - ISSN 0002-7863
Roč. 144, č. 28 (2022), s. 12725-12731Number of pages 7 s. Language eng - English Country US - United States Keywords nc-AFM ; on surface chemistry ; polymers Subject RIV BM - Solid Matter Physics ; Magnetism OECD category Condensed matter physics (including formerly solid state physics, supercond.) Subject RIV - cooperation J. Heyrovsky Institute of Physical Chemistry - Physical ; Theoretical Chemistry R&D Projects GX20-13692X GA ČR - Czech Science Foundation (CSF) GJ19-13126Y GA ČR - Czech Science Foundation (CSF) Research Infrastructure CzechNanoLab - 90110 - Vysoké učení technické v Brně Method of publishing Open access Institutional support FZU-D - RVO:68378271 ; UFCH-W - RVO:61388955 UT WOS 000829574800001 EID SCOPUS 85134720574 DOI 10.1021/jacs.2c02700 Annotation Here, we present a combined strategy toward the fabrication of one-dimensional porphyrinoid-based polymers homocoupled via surface-catalyzed [3 + 3] cycloaromatization of isopropyl substituents on Au(111). Scanning tunneling microscopy and noncontact atomic force microscopy describe the thermal-activated intra- and intermolecular oxidative ring closure reactions as well as the controlled tip-induced hydrogen dissociation from the porphyrinoid units.
Workplace Institute of Physics Contact Kristina Potocká, potocka@fzu.cz, Tel.: 220 318 579 Year of Publishing 2023 Electronic address https://hdl.handle.net/11104/0333953
Number of the records: 1