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Terahertz dynamics of nanoconfined water molecules
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SYSNO ASEP 0486556 Document Type C - Proceedings Paper (int. conf.) R&D Document Type Conference Paper Title Terahertz dynamics of nanoconfined water molecules Author(s) Zhukova, E.S. (RU)
Belyanchikov, M. A. (RU)
Torgashev, V. I. (RU)
Thomas, V.G. (RU)
Savinov, Maxim (FZU-D) RID, ORCID
Kadlec, Christelle (FZU-D) RID, ORCID
Kadlec, Filip (FZU-D) RID, ORCID, SAI
Prokhorov, A. S. (RU)
Kadyrov, L.S. (RU)
Petzelt, Jan (FZU-D) RID, ORCID, SAI
Ostapchuk, Tetyana (FZU-D) RID, ORCID
Fursenko, D.A. (RU)
Thomas, P.V. (RU)
Shakurov, G.S. (RU)
Dressel, M. (DE)
Gorshunov, B. (RU)Number of authors 16 Article number 7758778 Source Title Proceedings of the 41st International Conference on Infrared, Millimeter and Terahertz Waves - IRMMW-THz 2016. - New York : IEEE, 2016 - ISSN 2162-2027 - ISBN 978-146738485-8 Pages s. 1-2 Number of pages 2 s. Publication form Online - E Action 41st International Conference on Infrared, Millimeter and Terahertz Waves Event date 25.09.2016 - 30.09.2016 VEvent location Copenhagen Country DK - Denmark Event type WRD Language eng - English Country US - United States Keywords terahertz ; water molecules ; ferroelectric ; infrared Subject RIV BM - Solid Matter Physics ; Magnetism OECD category Condensed matter physics (including formerly solid state physics, supercond.) Institutional support FZU-D - RVO:68378271 UT WOS 000391406200439 EID SCOPUS 85006164580 DOI 10.1109/IRMMW-THz.2016.7758778 Annotation We performed spectroscopic studies of watercontaining beryl crystals. At terahertz frequencies, we observed a strongly temperature-dependent spectral feature, corresponding to a collective excitation caused by dipole-dipole interactions between separate H2O molecules. We associate the excitation with a soft mode signaling an incipient ferroelectric state within the water molecular subsystem. Single-particle excitations of nanocaged H2O molecules are also observed at terahertz and infrared frequencies using DFT analysis, their origin is assigned to translational and librational vibrational states.
Workplace Institute of Physics Contact Kristina Potocká, potocka@fzu.cz, Tel.: 220 318 579 Year of Publishing 2018
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