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Interactions between vibrational polyads of propyne, H3C-C-CH: Rotational and rovibrational spectroscopy of the levels around 1000 cm(-1)

  1. 1.
    SYSNO ASEP0336503
    Document TypeJ - Journal Article
    R&D Document TypeJournal Article
    Subsidiary JČlánek ve WOS
    TitleInteractions between vibrational polyads of propyne, H3C-C-CH: Rotational and rovibrational spectroscopy of the levels around 1000 cm(-1)
    Author(s) Pracna, Petr (UFCH-W)
    Müller, H. S. P. (DE)
    Urban, Š. (CZ)
    Horneman, V. M. (FI)
    Klee, S. (DE)
    Source TitleJournal of Molecular Spectroscopy. - : Elsevier - ISSN 0022-2852
    Roč. 256, č. 1 (2009), s. 152-162
    Number of pages11 s.
    Languageeng - English
    CountryUS - United States
    Keywordsmethylacetylene ; high resolution ; FTIR spectroscopy
    Subject RIVCF - Physical ; Theoretical Chemistry
    R&D ProjectsIAA400400706 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR)
    IAA400400504 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR)
    LC06071 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    CEZAV0Z40400503 - UFCH-W (2005-2011)
    UT WOS000268400600024
    DOI https://doi.org/10.1016/j.jms.2009.04.003
    AnnotationThe study of vibration resonance physics in propyne is based on experimental measurements of about 600 new rotational transitions between 495–590 and 700–760 GHz in excited vibrational levels v5 = 1, v8 = 1, v10 = 3 and v9 = v10 = 1 with vibrational energies around 1000 cm–1. The limits to the assignments and analysis were imposed by as yet unresolved anharmonic resonances with the states of the next higher polyad of levels lying above 1200 cm–1, which affect the rotational states involved in transitions that would be measurable with non-vanishing intensities. Vibration-rotation spectra pertaining to the levels in question were studied in the regions 880–1150 cm–1 (the v5 and v8 fundamental bands), 550–750 cm–1 (the v9 = v10 = 1 <- v10 = 1 hot bands) and 250–400 cm–1 (the v10 = 3 <- v10 = 2 “superhot” bands). A simultaneous least-squares fit of both types of data provides their reliable but in the case of accurate rotational data not always fully quantitative reproduction.
    WorkplaceJ. Heyrovsky Institute of Physical Chemistry
    ContactMichaela Knapová, michaela.knapova@jh-inst.cas.cz, Tel.: 266 053 196
    Year of Publishing2012
Number of the records: 1  

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