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Utilizing constant energy difference between sp-peak and C 1s core level in photoelectron spectra for unambiguous identification and quantification of diamond phase in nanodiamonds

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    SYSNO ASEP0584934
    Document TypeJ - Journal Article
    R&D Document TypeJournal Article
    Subsidiary JČlánek ve WOS
    TitleUtilizing constant energy difference between sp-peak and C 1s core level in photoelectron spectra for unambiguous identification and quantification of diamond phase in nanodiamonds
    Author(s) Romanyuk, Olexandr (FZU-D) RID, ORCID
    Stehlík, Štěpán (FZU-D) RID, ORCID
    Zemek, Josef (FZU-D) RID, ORCID
    Aubrechtová Dragounová, Kateřina (FZU-D) ORCID
    Kromka, Alexander (FZU-D) RID, ORCID, SAI
    Number of authors5
    Article number590
    Source TitleNanomaterials. - : MDPI - ISSN 2079-4991
    Roč. 14, č. 7 (2024)
    Number of pages14 s.
    Languageeng - English
    CountryCH - Switzerland
    Keywordsnanodiamond ; XPS ; UPS ; Raman spectroscopy ; graphitization ; ArCIB sputtering
    Subject RIVBM - Solid Matter Physics ; Magnetism
    OECD categoryCondensed matter physics (including formerly solid state physics, supercond.)
    R&D ProjectsLM2023051 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    LUASK22202 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    EH22_008/0004596 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    LUASK22147 GA MŠMT - Ministry of Education, Youth and Sports (MEYS)
    Method of publishingOpen access
    Institutional supportFZU-D - RVO:68378271
    UT WOS001201668000001
    EID SCOPUS85190278398
    DOI https://doi.org/10.3390/nano14070590
    AnnotationWe conducted a comparative analysis of the graphitization process in various types of hydrogenated NDs, considering differences in ND size and quality. The samples underwent annealing in an ultra-high vacuum and sputtering by Ar cluster ion beam (ArCIB). Samples were investigated by in situ X-ray photoelectron spectroscopy (XPS), in situ ultraviolet photoelectron spectroscopy (UPS), and Raman spectroscopy (RS). Our investigation revealed that the graphitization temperature of NDs ranges from 600 °C to 700 °C and depends on the size and crystallinity of the NDs. We revealed a constant energy difference of 271.3 eV between the sp-peak in the valence band spectra (at around 13.7 eV) and the sp3 component in the C 1s core level spectra (at 285.0 eV). The identification of this energy difference helps in calibrating charge shifts and serves the unambiguous identification of the sp3 bond contribution in the C 1s spectra obtained from ND samples.
    WorkplaceInstitute of Physics
    ContactKristina Potocká, potocka@fzu.cz, Tel.: 220 318 579
    Year of Publishing2025
    Electronic addresshttps://hdl.handle.net/11104/0352710
Number of the records: 1  

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