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Ultra-broad-band dielectric spectroscopy and phonons in (Pb.sub.1-x/2./sub.La.sub.x./sub.)(Zr.sub.0.9./sub.Ti.sub.0.1./sub.)O.sub.3./sub..
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SYSNO ASEP 0352316 Document Type J - Journal Article R&D Document Type Journal Article Subsidiary J Článek ve WOS Title Ultra-broad-band dielectric spectroscopy and phonons in (Pb1-x/2Lax)(Zr0.9Ti0.1)O3. Author(s) Buixaderas, Elena (FZU-D) RID, ORCID
Bovtun, Viktor (FZU-D) RID, ORCID, SAI
Veljko, Sergiy (FZU-D)
Savinov, Maxim (FZU-D) RID, ORCID
Kužel, Petr (FZU-D) RID, ORCID, SAI
Gregora, Ivan (FZU-D) RID, ORCID
Kamba, Stanislav (FZU-D) RID, ORCID, SAI
Reaney, I. (GB)Source Title Journal of Applied Physics. - : AIP Publishing - ISSN 0021-8979
Roč. 108, č. 10 (2010), 104101/1-104101/10Number of pages 10 s. Language eng - English Country US - United States Keywords PLZT ; phase transitions ; Raman and IR spectroscopy ; ferro-antiferroelectricity Subject RIV BM - Solid Matter Physics ; Magnetism R&D Projects KAN301370701 GA AV ČR - Academy of Sciences of the Czech Republic (AV ČR) GAP204/10/0616 GA ČR - Czech Science Foundation (CSF) CEZ AV0Z10100520 - FZU-D (2005-2011) UT WOS 000285005000108 DOI 10.1063/1.3501105 Annotation The dielectric behavior of (Pb1−x/2Lax)(Zr0.9Ti0.1)O3 PLZT 100x/90/10 (0 ≤ 100x ≤ 1) was studied in the frequency range 102–1014 Hz using dielectric, time-domain terahertz (THz), far-infrared, and Raman spectroscopy in the temperature interval 10–900 K. PZT 90/10 and PLZT 2/90/10 undergo two phase transitions, from a cubic paraelectric to a rhombohedral untilted ferroelectric (FE) phase and on further cooling to a tilted FE phase. PLZT 4/90/10 and PLZT 10/90/10 are incommensurately modulated and composed of an intergrowth of polar and antipolar cation displacements. These samples consequently demonstrate a FE soft mode which exhibits minimal frequency several tens of degrees above the nominal antiferroelectric phase transition temperature. The dielectric response of PLZT 100x/90/10 is mainly governed by a gigahertz relaxation and a soft phonon component in the THz range. Workplace Institute of Physics Contact Kristina Potocká, potocka@fzu.cz, Tel.: 220 318 579 Year of Publishing 2011
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