Overview of S(T)EM electron detectors with garnet scintillators: Some potentials and limits

0544784 - ÚPT 2022 RIV US eng J - Journal Article
Schauer, Petr - Lalinský, Ondřej - Kučera, M.
Overview of S(T)EM electron detectors with garnet scintillators: Some potentials and limits.
Microscopy Research and Technique. Roč. 84, č. 4 (2021), s. 753-770. ISSN 1059-910X. E-ISSN 1097-0029
R&D Projects: GA MPO(CZ) FV30271; GA MŠMT(CZ) LO1212; GA MŠMT ED0017/01/01
Institutional support: RVO:68081731
Keywords : cathodoluminescence * conductive coating * garnet film scintillator * light guide * SEM electron detector
OECD category: Electrical and electronic engineering
Impact factor: 2.893, year: 2021
Method of publishing: Open access
https://analyticalsciencejournals.onlinelibrary.wiley.com/doi/10.1002/jemt.23634

The paper is focused on a complete configuration and design of a scintillation electron detector in scanning electron and/or scanning transmission electron microscopes (S(T)EM) with garnet scintillators. All processes related to the scintillator and light guide were analyzed. In more detail, excitation electron trajectories and absorbed energy distributions, efficiencies and kinetics of scintillators, as well as the influence of their anti-charging coatings and their substrates, assigned optical properties, and light guide efficiencies of different configurations were presented and discussed. The results indicate problems with low-energy detection below 1 keV when the scandium conductive coating with a thickness of only 3 nm must be used to allow electron penetration without significant losses. It was shown that the short rise and decay time and low afterglow of LuGdGaAG:Ce liquid-phase epitaxy garnet film scintillators guarantee a strong modulation transfer function of the entire imaging system resulting in a contrast transfer ability up to 0.6 lp/pixel. Small film scintillator thicknesses were found to be an advantage due to the low signal self-absorption. The optical absorption coefficients, refractive indices, and the mirror optical reflectance of materials involved in the light transport to the photomultiplier tube photocathode were investigated. The computer-optimized design SCIUNI application was used to configure the optimized light guide system. It was shown that nonoptimized edge-guided systems possess very poor light guiding efficiency as low as 1%, while even very complex optimized ones can achieve more than 20%.
Permanent Link: http://hdl.handle.net/11104/0321592