Issue 42, 2022

Formation of spin-polarized current in antiferromagnetic polymer spintronic field-effect transistors

Abstract

We have theoretically investigated the feasibility of constructing a spintronic field-effect transistor with the active channel made of a polymer chain with the antiferromagnetic coupling oriented in the source-to-drain direction. We found two different device function regimes controlling the on-chain spin–charge carrier density by tuning the gate voltage. At higher charge carrier densities, the source–drain current linearly increases with decreasing charge carrier densities. In this regime, no polymer spin-polarized current is observed. Upon reaching a critical gate voltage, the current decreases with decreasing charge densities. It is accompanied by the formation of spin-polarized current, generated by an on-chain process, which can be related to spin–charge spatial distribution symmetry breaking caused either by an application of the source-to-drain voltage (higher spin polarization near the drain), or the breakdown of the Peierls dimerization near chain ends. Numerical simulation of the transistor characteristics suggests that the design of a polymer spintronic field-effect transistor is in principle feasible.

Graphical abstract: Formation of spin-polarized current in antiferromagnetic polymer spintronic field-effect transistors

Article information

Article type
Paper
Submitted
08 Jul 2022
Accepted
27 Sep 2022
First published
27 Sep 2022

Phys. Chem. Chem. Phys., 2022,24, 25999-26010

Formation of spin-polarized current in antiferromagnetic polymer spintronic field-effect transistors

S. Sun, M. Menšík, C. Ganzorig, P. Toman and J. Pfleger, Phys. Chem. Chem. Phys., 2022, 24, 25999 DOI: 10.1039/D2CP03119A

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